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2018 Aggregate frequency width, nuclear hyperfine coupling and Jahn–Teller effect of Cu2+ impurity ion ESR in SrLaAlO4 dielectric resonator at 20 millikelvin

发布时间:2018-02-23          来源:           浏览次数:

M A Hosain1 , J-M Le Floch1,2, J Krupka3 and M E Tobar1
1 ARC Centre of Excellence for Engineered Quantum Systems, School of Physics, University of Western
Australia, 35 Stirling Highway, Crawley WA 6009, Australia
2 MOE Key Laboratory of Fundamental Physical Quantities Measurement, School of Physics, Huazhong
University of Science and Technology, Wuhan 430074, Hubei, People’s Republic of China
3 Department of Electronics and Information Technology, Institute of Microelectronics
and Optoelectronics, Warsaw University of Technology, Koszykowa 75, 00-662 Warszawa, Poland

The impurity paramagnetic ion, Cu2+ substitutes Al in the SrLaAlO4 single crystal lattice, this results in a CuO6 elongated octahedron, and the resulting measured g-factors satisfy four-fold axes variation condition. The aggregate frequency width of the electron spin
resonance with the required minimum level of impurity concentration has been evaluated in this single crystal SrLaAlO4 at 20 millikelvin. Measured parallel hyperfine constants, ACu, were determined to be −155.7 × 10−4 cm−1, − 163.0 × 10−4 cm−1, − 178.3 × 10−4 cm−1 and −211.1 × 10−4 cm−1 at 9.072 GHz (WGH4,1,1) for the nuclear magnetic quantum number MI = +3/2,+1/2,−1/2, and−3/2 respectively. The anisotropy of the hyperfine structure reveals the characteristics of the static Jahn–Teller effect. The second-order-anisotropy term, ~( spin−orbit coupling/10Dq)2, is significant and cannot be disregarded, with the local strain dominating over the observed Zeeman-anisotropy-energy difference. The Bohr electron magneton, = 9.23 × 1024JT−1, (within −0.43% so-called experimental error) has been found using the measured spin-Hamiltonian parameters. Measured nuclear dipolar hyperfine structure parameter P = 12.3 × 10−4 cm−1 shows that the mean inverse third power of the electron distance from the nucleus is rq−3 ~= 5.23 a.u. for Cu2+ ion in the substituted Al3+ ion site assuming nuclear electric quadruple moment Q = −0.211 barn.


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